... but I do not understand why it is less economical than the Mk 3 at speeds over 60 mph...
Unfortunately I'm unfamiliar with the MK3 (or any of its predecessors)! - The MK4 facelift is my first Honda (probably not my last)
However, I also found the MK4 to be optimized for speeds up to little above 50 mph (80 to 100 km/h).
So far I was unable to get official information about relevant data like drag coefficient and/or front area for newer Jazz models. (My assumptions so far involve a drag coefficient around 0.32 and a front area of about 2.15 sqare meters - if anyone should have more accurate data, please don't hesitate to PM me! - thank you!)
As we all know, air drag increases
exponentially with speed (and the Jazz - for all its benefits - doesn't qualify exactly as a "lean, low-build sportscar"

- so, it is alone from its build at a disadvantage.
Please do correct me, if I should have gotten this wrong!
From what Wikipedia tells about the Jazz MK3: It never was offered as a "hybrid" but only as a "normal" petrol car.
This changes things enormously fuel-efficency-wise:
- a "normal" car with petrol engine absolutely sucks in low-demand situations like city stop-and-go traffic
- a "normal" car with petrol engine will "shine" during high load conditions (like motorway travel at higher speeds)
Now enter the Jazz MK4 hybrid:
- as you have already found out: It absolutely "thrives" in the city!
- it is a worthy contestant on A-roads
- it literally "sucks" at motorway speeds (even more so above!)
It all boils down to this: The Jazz's e:HEV system was built and optimized for low(er) speed situations.
If your driving profile should mainly consist of high(er) speed motoring, you will absolutely be disapointed by the Jazz's mpg!
(and - imho: you just might have bought the wrong car for your needs)